The operator Schmidt rank of an operator acting on the tensor product Cⁿ⊗C^m is the number of terms in a decomposition of the operator as a sum of simple tensors with factors forming orthogonal families in their respective matrix algebras. It has been known that for unitary operators acting on two copies of C², the operator Schmidt rank can only take the values 1, 2, and 4, the value 3 being forbidden. In this paper, we settle an open question, showing that the above obstruction is the only one occurring. We do so by constructing explicit examples of bipartite unitary operators of all possible operator Schmidt ranks, for arbitrary dimensions (n,m)≠(2,2).